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The Sweater of Tears is a sweater that appears in the episode "Dying for Pie" and is one out of two sweaters seen in the episode.
As the name states, it is a sweater made entirely of SpongeBob's tears.
After the eyelash sweater SpongeBob makes for Squidward in honor of Employee Brotherhood Day fails to please him, this upsets the former and leads him to creating a sweater made of his tears, asking Squidward if he likes it any better.
The sweater is also mentioned later in the episode when Mr. Krabs complains to Squidward that SpongeBob cried him a sweater of tears and he just had to kill him with an Exploding Pie (which later turns out to have been in the latter's pocket the whole time, meaning he didn't actually eat it).